trying to get to a no-till situation where there is always a layer of mulch, or ramial chips, or cover crop.
I would like more details if possible. For what this land will be used? What you want to do there. Food forest? Vegetable garden?
As you said, if you only want no-till situation, layer of mulch, or ramial chips, or cover crop you already have all this. Mulch will be always available by cutting the vegetation and other woody stuff growing there.
For cover crop. Take some soil and mix in the rye seeds. Add water to get muddy liquid. Add more soil so the stuff is not muddy any more. Broadcast. From here on cover crop will be always there, self seeding every year if you don't harvest. You just need to cut everything in october for best results or you could leave it to nature.
As Paul said, rye will not suppress your "weeds".
Why not use bramble as food? It grows from one main root. In winter cut and weed the area, leaving one or two main strongest shoots from these roots. Hang them to a 3-4 meter pole with a hook on the end. Plenty of fruit.