I love moss and think this is a great idea! I bet spring ephemerals could be a good fit in such a guild since they only exist for a short time and usually want similar conditions to moss. I've seen Sweet Cicely (Osmorhiza claytonii) growing with moss in their understory. Since their habit is more upright, they allow space underneath. There's a guild in my
yard of Cup Plant, Chickweed, Sweet Cicely and many others where moss grows in the understory. I didn't plant this guild, but it does amazingly well. Elderberry or similar could be a good possibility for a larger plant in the mix. Wild Ginger might work, though it can spread quite a bit and might be too aggressive, not sure. Looking forward to what ideas other folks might have! When I have the time, I might have to reread Gathering Moss by Robin Wall Kimmerer to see if that yields any ideas.
“Action on behalf of life transforms. Because the relationship between self and the world is reciprocal, it is not a question of first getting enlightened or saved and then acting. As we work to heal the earth, the earth heals us.” ~ Robin Wall Kimmerer